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The government told the Iranian nuclear agency to begin work on five sites, with five more to be located over the next two months.
It comes days after the UN nuclear watchdog rebuked Iran for covering up a uranium enrichment plant.
The White House said the move was "yet another serious violation of Iran's clear obligations".
Meanwhile, Britain described the news as "a matter of serious concern" and potentially a "deliberate breach" of UN resolutions.
President Ahmadinejad is also calling for his cabinet to approve a move to increase the enrichment to 20%, up from 5%.