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There are a variety of different ways to start the synchronicity between Dark Side of the Moon and Wizard of Oz. Conventional knowledge seems to hold that the famed Third Roar Theory is the best of the bunch, but I leave it up to you to experiment and choose your own favorite.
Third Roar Theory
Perhaps the best known variation of the Dark Side of the Rainbow synchronicity is the Third Roar Theory. It's certainly the first variation I myself discovered. It works very well and is relatively easy to set up. First put in cd, tape, or record of Dark Side of the Moon that you're going to use; generally this is easiest with cd, but if you're "slumming" it, it is possible to do it with other media (although considerably more difficult).
Originally posted by Karlhungis
Dark Side of the Moon is probably my favorite album of all time. I just think that Pink Floyd is its own category. I don't think of it as rock.