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"When you first meet Ultron, his physicality is very different to what he evolves to. It was in the script but we arrived at the metamorphosis of him on the set. In practice, in rehearsals ... We were able to create the physicality of the character on the motion-capture stage. They would dot me up and I was wearing a helmet that had two cameras on my face, and they could live stream it to a monitor so we could try different things. Then I'd go and shoot the scene with the other actors and they're recording all of it, including my voice. 9 times out of 10 they were not using ADR (additional dialogue recording) after the fact."
I grew up reading the comic-book version and I imagined Ultron speaking in an electronic voice.