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Character actor Wallach - who began his film career in 1956 after 10 years on stage - was admired for his wide range in a career spanning six decades.
His portrayal of bandit chief Calvera in The Magnificent Seven was regarded by many as his definitive role.
When he received an honorary Oscar in 2011, he was described as a "quintessential chameleon".
Though he was never nominated for an Oscar during his 60-year career, the Academy rewarded him in 2011 for "effortlessly inhabiting a wide range of characters, while putting his inimitable stamp on every role".